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Preheat oven to 425°F. In a large bowl, combine Brussels sprouts, orange zest, a pinch of salt and a few hefty grinds of pepper. Toss to combine. Drizzle with olive oil and toss again.
Spread Brussels sprouts mixture on a foil-lined baking sheet. Roast until bright and golden, 20 to 25 minutes. Transfer to a serving bowl and spritz with orange wedges to serve.